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Capacitance response and concentration fluctuations close to ionic liquid-solvent demixing
(Elsevier, 2022-01)
We investigate the concentration fluctuations in a simple model of electrolyte (two positively and negatively charged Lennard-Jones spheres in a solution of an uncharged Lennard-Jones liquid) confined between electrodes ...
Capillary Ionization and Jumps of Capacitive Energy Stored in Mesopores
(American Chemical Society, 2021-04-30)
We study ionic liquid–solvent mixtures in slit-shaped nanopores wider than a few ion diameters. Using a continuum theory and generic thermodynamic reasoning, we reveal that such systems can undergo a capillary ionization ...
Effect of proximity to ionic liquid-solvent demixing on electrical double layers
(Journal of Molecular Liquids, 2019-11)
There is a growing interest in the properties of ionic liquids (ILs) and IL-solvent mixtures at metallic interfaces, particularly due to their applications in energy storage. The main focus so far has been on electrical ...
Electrical Double Layers Close to Ionic Liquid–Solvent Demixing
(American Chemical Society, 2018-12-31)
Electrical double layers (EDLs) play a key role in energy storage and have been suggested to have applications in energy generation. Recently, there has been an expansion of interest in EDLs, but EDLs with ionic liquid–solvent ...